Advances in Catalysis and Related Subjects, Volume 9 by W G Frankenberg

By W G Frankenberg

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24. Barton, D. H. , Cookson, R. , and Shoppee, C. , Chemistry & Industry p. 21 (1954). 26. Corey, E. , and Sneen, R. , J. A m . Chem. 7 7 , 2505 (1955). 5 The Reaction of Hydrogen and Ethylene on Several Faces of a Single Crystal of Nickel ROBERT E. CUNNINGHAM AND ALL,AN T. The (321) face had the fastest rate and the (100) face the slowest rate in all cases, the maximum difference being approximately tenfold. The relative reaction rates could not be explained on the basis of simple crystal geometry.

Physik. Chem. 289-316 (1924) ; Chem. Abstr. 23,2872 (1929). 6 . Beckett, C. , Pitzer, K . , and Spitzer, R. , J . Am. Chem. 69. 2188 (1947). 7. Signaigo, F. , and Cramer, P. , J . Am. Chem. 66,3326 (1933). 8 . Bailey, W. J . , Hewitt, J. J . , J. Am. Chem. Soc. 77, 357 (1955). 9. , Ph. D. dissertation, Department of Chemistry, University of Arkansas, 1956. To be available on microfilm from University Microfilms, Ann Arbor, Michigan. 10. Hammond, G. , and Nevitt, T. , J . Am. Chem. 76, 4121 (1954).

For the problem a t hand, this type of study has revealed that the principal product of the hydrogenation of an unsaturated compound is formed by the addition of two atoms of hydrogen to the same side of the molecule. This is deduced from the formation of cis olefins from disubstituted acetylenes and meso-1 ,2-dimethylsuccinicacid from dimethylmaleic acid ( I ) . *This work was supported by a generous grant from the Petroleum Research Fund of the American Chemical Society. Graduate Fellow under the American Chemical Society Petroleum Research Fund, 1954-1956.

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